APM OpenIR
Mobile Ions in Composite Solids
Zou, Zheyi1; Li, Yajie1; Lu, Ziheng2; Wang, Da1; Cui, Yanhua4; Guo, Bingkun5; Li, Yuanji1; Liang, Xinmiao6; Feng, Jiwen6; Li, Hong7; Nan, Ce-Wen8; Armand, Michel9; Chen, Liquan7; Xu, Kang3; Shi, Siqi1
2020-05-13
Source PublicationCHEMICAL REVIEWS
ISSN0009-2665
Volume120Issue:9Pages:4169-4221
AbstractFast ion conduction in solid-state matrices constitutes the foundation for a wide spectrum of electrochemical systems that use solid electrolytes (SEs), examples of which include solid-state batteries (SSBs), solid oxide fuel cells (SOFCs), and diversified gas sensors. Mixing different solid conductors to form composite solid electrolytes (CSEs) introduces unique opportunities for SEs to possess exceptional overall performance far superior to their individual parental solids, thanks to the abundant chemistry and physics at the new interfaces thus created. In this review, we provide a comprehensive and in-depth examination of the development and understanding of CSEs for SSBs, with special focus on their physiochemical properties and mechanisms of ion transport therein. The origin of the enhanced ionic conductivity in CSEs relative to their single-phase parents is discussed in the context of defect chemistry and interfacial reactions. The models/theories for ion movement in diversified composites are critically reviewed to interrogate a general strategy to the design of novel CSEs, while properties such as mechanical strength and electrochemical stability are discussed in view of their perspective applications in lithium metal batteries and beyond. As an integral component of understanding how ions interact with their composite environments, characterization techniques to probe the ion transport kinetics across different temporal and spatial time scales are also summarized.
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Basic Research Program of Shenzhen ; Basic Research Program of Shenzhen ; Shanghai Pujiang Program ; Shanghai Pujiang Program ; Shanghai Sailing Program ; Shanghai Sailing Program ; Open Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Open Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Shanghai Engineering Research Center of Intelligent Computing System ; Shanghai Engineering Research Center of Intelligent Computing System ; Joint Center of Energy Storage Research (JCESR), an energy hub - US Department of Energy Office of Science ; Joint Center of Energy Storage Research (JCESR), an energy hub - US Department of Energy Office of Science ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Basic Research Program of Shenzhen ; Basic Research Program of Shenzhen ; Shanghai Pujiang Program ; Shanghai Pujiang Program ; Shanghai Sailing Program ; Shanghai Sailing Program ; Open Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Open Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Shanghai Engineering Research Center of Intelligent Computing System ; Shanghai Engineering Research Center of Intelligent Computing System ; Joint Center of Energy Storage Research (JCESR), an energy hub - US Department of Energy Office of Science ; Joint Center of Energy Storage Research (JCESR), an energy hub - US Department of Energy Office of Science ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Basic Research Program of Shenzhen ; Basic Research Program of Shenzhen ; Shanghai Pujiang Program ; Shanghai Pujiang Program ; Shanghai Sailing Program ; Shanghai Sailing Program ; Open Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Open Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Shanghai Engineering Research Center of Intelligent Computing System ; Shanghai Engineering Research Center of Intelligent Computing System ; Joint Center of Energy Storage Research (JCESR), an energy hub - US Department of Energy Office of Science ; Joint Center of Energy Storage Research (JCESR), an energy hub - US Department of Energy Office of Science ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Basic Research Program of Shenzhen ; Basic Research Program of Shenzhen ; Shanghai Pujiang Program ; Shanghai Pujiang Program ; Shanghai Sailing Program ; Shanghai Sailing Program ; Open Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Open Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Shanghai Engineering Research Center of Intelligent Computing System ; Shanghai Engineering Research Center of Intelligent Computing System ; Joint Center of Energy Storage Research (JCESR), an energy hub - US Department of Energy Office of Science ; Joint Center of Energy Storage Research (JCESR), an energy hub - US Department of Energy Office of Science
DOI10.1021/acs.chemrev.9b00760
WOS KeywordSTATE LITHIUM BATTERIES ; SPACE-CHARGE REGIONS ; LI-AIR BATTERIES ; NANOCOMPOSITE POLYMER ELECTROLYTES ; ACCELERATED MOLECULAR-DYNAMICS ; ELECTROCHEMICAL PROPERTIES ; POLY(ETHYLENE OXIDE) ; CONDUCTIVITY ENHANCEMENT ; ELECTRICAL-CONDUCTIVITY ; GLASS-CERAMICS
Language英语
Funding ProjectNational Natural Science Foundation of China[U1630134] ; National Natural Science Foundation of China[U1930208] ; National Natural Science Foundation of China[51622207] ; National Natural Science Foundation of China[51802187] ; National Natural Science Foundation of China[11874254] ; Basic Research Program of Shenzhen[JCYJ20190812161409163] ; Shanghai Pujiang Program[2019PJD016] ; Shanghai Sailing Program[18YF1408700] ; Open Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China[SKLASS2018-01] ; Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China[SKLASS2019-Z023] ; Shanghai Engineering Research Center of Intelligent Computing System[19DZ2252600] ; Joint Center of Energy Storage Research (JCESR), an energy hub - US Department of Energy Office of Science[IAA SN2020957]
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Basic Research Program of Shenzhen ; Basic Research Program of Shenzhen ; Shanghai Pujiang Program ; Shanghai Pujiang Program ; Shanghai Sailing Program ; Shanghai Sailing Program ; Open Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Open Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Shanghai Engineering Research Center of Intelligent Computing System ; Shanghai Engineering Research Center of Intelligent Computing System ; Joint Center of Energy Storage Research (JCESR), an energy hub - US Department of Energy Office of Science ; Joint Center of Energy Storage Research (JCESR), an energy hub - US Department of Energy Office of Science ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Basic Research Program of Shenzhen ; Basic Research Program of Shenzhen ; Shanghai Pujiang Program ; Shanghai Pujiang Program ; Shanghai Sailing Program ; Shanghai Sailing Program ; Open Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Open Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Shanghai Engineering Research Center of Intelligent Computing System ; Shanghai Engineering Research Center of Intelligent Computing System ; Joint Center of Energy Storage Research (JCESR), an energy hub - US Department of Energy Office of Science ; Joint Center of Energy Storage Research (JCESR), an energy hub - US Department of Energy Office of Science ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Basic Research Program of Shenzhen ; Basic Research Program of Shenzhen ; Shanghai Pujiang Program ; Shanghai Pujiang Program ; Shanghai Sailing Program ; Shanghai Sailing Program ; Open Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Open Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Shanghai Engineering Research Center of Intelligent Computing System ; Shanghai Engineering Research Center of Intelligent Computing System ; Joint Center of Energy Storage Research (JCESR), an energy hub - US Department of Energy Office of Science ; Joint Center of Energy Storage Research (JCESR), an energy hub - US Department of Energy Office of Science ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Basic Research Program of Shenzhen ; Basic Research Program of Shenzhen ; Shanghai Pujiang Program ; Shanghai Pujiang Program ; Shanghai Sailing Program ; Shanghai Sailing Program ; Open Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Open Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Project of the State Key Laboratory of Advanced Special Steel, Shanghai University, China ; Shanghai Engineering Research Center of Intelligent Computing System ; Shanghai Engineering Research Center of Intelligent Computing System ; Joint Center of Energy Storage Research (JCESR), an energy hub - US Department of Energy Office of Science ; Joint Center of Energy Storage Research (JCESR), an energy hub - US Department of Energy Office of Science
WOS Research AreaChemistry
WOS SubjectChemistry, Multidisciplinary
WOS IDWOS:000535249500006
PublisherAMER CHEMICAL SOC
Citation statistics
Cited Times:5[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.apm.ac.cn/handle/112942/22746
Collection中国科学院武汉物理与数学研究所
Corresponding AuthorLi, Yajie; Lu, Ziheng; Wang, Da; Xu, Kang; Shi, Siqi
Affiliation1.Shanghai Univ, Sch Mat Sci & Engn, State Key Lab Adv Special Steel, Shanghai 200444, Peoples R China
2.Chinese Acad Sci, Shenzhen Inst Adv Technol, Shenzhen 518055, Peoples R China
3.US Army, Res Lab, Energy Storage Branch, Energy & Biotechnol Div,Sensor & Elect Directorat, Adelphi, MD 20783 USA
4.China Acad Engn Phys, Inst Elect Engn, Mianyang 621000, Sichuan, Peoples R China
5.Shanghai Univ, Mat Genome Inst, Shanghai 200444, Peoples R China
6.Chinese Acad Sci, Wuhan Inst Phys & Math, Wuhan 430071, Peoples R China
7.Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China
8.Tsinghua Univ, Sch Mat Sci & Engn, Beijing 100084, Peoples R China
9.CIC Energigune, Elect Energy Storage Dept, Parque Technol Alava, E-01510 Minano, Alava, Spain
Recommended Citation
GB/T 7714
Zou, Zheyi,Li, Yajie,Lu, Ziheng,et al. Mobile Ions in Composite Solids[J]. CHEMICAL REVIEWS,2020,120(9):4169-4221.
APA Zou, Zheyi.,Li, Yajie.,Lu, Ziheng.,Wang, Da.,Cui, Yanhua.,...&Shi, Siqi.(2020).Mobile Ions in Composite Solids.CHEMICAL REVIEWS,120(9),4169-4221.
MLA Zou, Zheyi,et al."Mobile Ions in Composite Solids".CHEMICAL REVIEWS 120.9(2020):4169-4221.
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