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Combined ultrafast spectroscopic and TDDFT theoretical studies on dual fluorescence emissions promoted by ligand-to-metal charge transfer (LMCT) excited states of tungsten -containing organometallic complexes
Liang, Yue1; Guo, Yurong1; Wang, Ye3; Zhang, Song3; Pan, Yu2; Shi, Yanan1; Wang, Yanan1; Zhu, Lina1; Jin, Bing3; Sun, Yan1; Zhang, Bing2; Feng, Xia1; Yuan, Minghu3; Wang, Haiyuan1; Zhao, Guangjiu1
2020-06-01
Source PublicationCHEMICAL PHYSICS LETTERS
ISSN0009-2614
Volume748Pages:6
AbstractIn this work, we first designed and synthesized two tungsten-containing organometallic complexes MeNOON and MeNOOO with novel dual fluorescence emissions. Moreover, the combined femtosecond ultrafast spectroscopy and time-dependent density functional theory (TDDFT) method has been performed to investigate the excited-state dynamics of MeNOON and MeNOOO complexes. It is distinctly demonstrated that dual fluorescence emissions of tungsten-containing organometallic complexes are originated from the localized-on-ligand (LL) and ligand-to-metal charge transfer (LMCT) excited states, respectively. Furthermore, the ultrafast LMCT process has been measured by the femtosecond spectroscopy.
KeywordDual fluorescence Localized-on-ligand Ligand-to-metal charge transfer Tungsten-containing organometallic Excited state
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Tianjin University ; Tianjin University ; Open Research Funds of State Key Laboratory of Bioelectronics (Southeast University) ; Open Research Funds of State Key Laboratory of Bioelectronics (Southeast University) ; Frontier Science Project of the Knowledge Innovation Program of Chinese Academy of Sciences (CAS) ; Frontier Science Project of the Knowledge Innovation Program of Chinese Academy of Sciences (CAS) ; State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics (Wuhan Institute of Physics and Mathematics of Chinese Academy of Sciences) ; State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics (Wuhan Institute of Physics and Mathematics of Chinese Academy of Sciences) ; Project for Excellent Member of CAS Youth Innovation Promotion Association ; Project for Excellent Member of CAS Youth Innovation Promotion Association ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Tianjin University ; Tianjin University ; Open Research Funds of State Key Laboratory of Bioelectronics (Southeast University) ; Open Research Funds of State Key Laboratory of Bioelectronics (Southeast University) ; Frontier Science Project of the Knowledge Innovation Program of Chinese Academy of Sciences (CAS) ; Frontier Science Project of the Knowledge Innovation Program of Chinese Academy of Sciences (CAS) ; State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics (Wuhan Institute of Physics and Mathematics of Chinese Academy of Sciences) ; State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics (Wuhan Institute of Physics and Mathematics of Chinese Academy of Sciences) ; Project for Excellent Member of CAS Youth Innovation Promotion Association ; Project for Excellent Member of CAS Youth Innovation Promotion Association ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Tianjin University ; Tianjin University ; Open Research Funds of State Key Laboratory of Bioelectronics (Southeast University) ; Open Research Funds of State Key Laboratory of Bioelectronics (Southeast University) ; Frontier Science Project of the Knowledge Innovation Program of Chinese Academy of Sciences (CAS) ; Frontier Science Project of the Knowledge Innovation Program of Chinese Academy of Sciences (CAS) ; State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics (Wuhan Institute of Physics and Mathematics of Chinese Academy of Sciences) ; State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics (Wuhan Institute of Physics and Mathematics of Chinese Academy of Sciences) ; Project for Excellent Member of CAS Youth Innovation Promotion Association ; Project for Excellent Member of CAS Youth Innovation Promotion Association ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Tianjin University ; Tianjin University ; Open Research Funds of State Key Laboratory of Bioelectronics (Southeast University) ; Open Research Funds of State Key Laboratory of Bioelectronics (Southeast University) ; Frontier Science Project of the Knowledge Innovation Program of Chinese Academy of Sciences (CAS) ; Frontier Science Project of the Knowledge Innovation Program of Chinese Academy of Sciences (CAS) ; State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics (Wuhan Institute of Physics and Mathematics of Chinese Academy of Sciences) ; State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics (Wuhan Institute of Physics and Mathematics of Chinese Academy of Sciences) ; Project for Excellent Member of CAS Youth Innovation Promotion Association ; Project for Excellent Member of CAS Youth Innovation Promotion Association
DOI10.1016/j.cplett.2020.137396
WOS KeywordLIGHT-EMITTING-DIODES ; TIME-RESOLVED FLUORESCENCE ; PHOTOPHYSICAL PROPERTIES ; TRANSIENT ABSORPTION ; DYNAMICS ; DECAY
Language英语
Funding ProjectNational Natural Science Foundation of China[21573229] ; National Natural Science Foundation of China[21873068] ; National Natural Science Foundation of China[21422309] ; Tianjin University ; Open Research Funds of State Key Laboratory of Bioelectronics (Southeast University) ; Frontier Science Project of the Knowledge Innovation Program of Chinese Academy of Sciences (CAS) ; State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics (Wuhan Institute of Physics and Mathematics of Chinese Academy of Sciences) ; Project for Excellent Member of CAS Youth Innovation Promotion Association
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Tianjin University ; Tianjin University ; Open Research Funds of State Key Laboratory of Bioelectronics (Southeast University) ; Open Research Funds of State Key Laboratory of Bioelectronics (Southeast University) ; Frontier Science Project of the Knowledge Innovation Program of Chinese Academy of Sciences (CAS) ; Frontier Science Project of the Knowledge Innovation Program of Chinese Academy of Sciences (CAS) ; State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics (Wuhan Institute of Physics and Mathematics of Chinese Academy of Sciences) ; State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics (Wuhan Institute of Physics and Mathematics of Chinese Academy of Sciences) ; Project for Excellent Member of CAS Youth Innovation Promotion Association ; Project for Excellent Member of CAS Youth Innovation Promotion Association ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Tianjin University ; Tianjin University ; Open Research Funds of State Key Laboratory of Bioelectronics (Southeast University) ; Open Research Funds of State Key Laboratory of Bioelectronics (Southeast University) ; Frontier Science Project of the Knowledge Innovation Program of Chinese Academy of Sciences (CAS) ; Frontier Science Project of the Knowledge Innovation Program of Chinese Academy of Sciences (CAS) ; State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics (Wuhan Institute of Physics and Mathematics of Chinese Academy of Sciences) ; State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics (Wuhan Institute of Physics and Mathematics of Chinese Academy of Sciences) ; Project for Excellent Member of CAS Youth Innovation Promotion Association ; Project for Excellent Member of CAS Youth Innovation Promotion Association ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Tianjin University ; Tianjin University ; Open Research Funds of State Key Laboratory of Bioelectronics (Southeast University) ; Open Research Funds of State Key Laboratory of Bioelectronics (Southeast University) ; Frontier Science Project of the Knowledge Innovation Program of Chinese Academy of Sciences (CAS) ; Frontier Science Project of the Knowledge Innovation Program of Chinese Academy of Sciences (CAS) ; State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics (Wuhan Institute of Physics and Mathematics of Chinese Academy of Sciences) ; State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics (Wuhan Institute of Physics and Mathematics of Chinese Academy of Sciences) ; Project for Excellent Member of CAS Youth Innovation Promotion Association ; Project for Excellent Member of CAS Youth Innovation Promotion Association ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Tianjin University ; Tianjin University ; Open Research Funds of State Key Laboratory of Bioelectronics (Southeast University) ; Open Research Funds of State Key Laboratory of Bioelectronics (Southeast University) ; Frontier Science Project of the Knowledge Innovation Program of Chinese Academy of Sciences (CAS) ; Frontier Science Project of the Knowledge Innovation Program of Chinese Academy of Sciences (CAS) ; State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics (Wuhan Institute of Physics and Mathematics of Chinese Academy of Sciences) ; State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics (Wuhan Institute of Physics and Mathematics of Chinese Academy of Sciences) ; Project for Excellent Member of CAS Youth Innovation Promotion Association ; Project for Excellent Member of CAS Youth Innovation Promotion Association
WOS Research AreaChemistry ; Physics
WOS SubjectChemistry, Physical ; Physics, Atomic, Molecular & Chemical
WOS IDWOS:000531489900013
PublisherELSEVIER
Citation statistics
Document Type期刊论文
Identifierhttp://ir.apm.ac.cn/handle/112942/22651
Collection中国科学院武汉物理与数学研究所
Corresponding AuthorZhang, Song; Pan, Yu; Zhao, Guangjiu
Affiliation1.Tianjin Univ, Natl Demonstrat Ctr Expt Chem & Chem Engn Educ, Natl Virtual Simulat Expt Teaching Ctr Chem & Che, Sch Sci,Tianjin Key Lab Mol Optoelect Sci,Dept Ch, Tianjin 300354, Peoples R China
2.Dalian Univ Technol, Sch Petr & Chem Engn, State Key Lab Fine Chem, Panjin 124221, Peoples R China
3.Chinese Acad Sci, Wuhan Inst Phys & Math, State Key Lab Magnet Resonance & Atom & Mol Phys, Wuhan 430071, Peoples R China
Recommended Citation
GB/T 7714
Liang, Yue,Guo, Yurong,Wang, Ye,et al. Combined ultrafast spectroscopic and TDDFT theoretical studies on dual fluorescence emissions promoted by ligand-to-metal charge transfer (LMCT) excited states of tungsten -containing organometallic complexes[J]. CHEMICAL PHYSICS LETTERS,2020,748:6.
APA Liang, Yue.,Guo, Yurong.,Wang, Ye.,Zhang, Song.,Pan, Yu.,...&Zhao, Guangjiu.(2020).Combined ultrafast spectroscopic and TDDFT theoretical studies on dual fluorescence emissions promoted by ligand-to-metal charge transfer (LMCT) excited states of tungsten -containing organometallic complexes.CHEMICAL PHYSICS LETTERS,748,6.
MLA Liang, Yue,et al."Combined ultrafast spectroscopic and TDDFT theoretical studies on dual fluorescence emissions promoted by ligand-to-metal charge transfer (LMCT) excited states of tungsten -containing organometallic complexes".CHEMICAL PHYSICS LETTERS 748(2020):6.
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