APM OpenIR
Solid-state NMR for metal-containing zeolites: From active sites to reaction mechanism
Zhao, Xingling1,2; Xu, Jun1,3; Deng, Feng1
2020-04-01
Source PublicationFRONTIERS OF CHEMICAL SCIENCE AND ENGINEERING
ISSN2095-0179
Volume14Issue:2Pages:159-187
AbstractMetal-containing zeolite catalysts have found a wide range of applications in heterogeneous catalysis. To understand the nature of metal active sites and the reaction mechanism over such catalysts is of great importance for the establishment of structure-activity relationship. The advanced solid-state NMR (SSNMR) spectroscopy is robust in the study of zeolites and zeolite-catalyzed reactions. In this review, we summarize recent developments and applications of SSNMR for exploring the structure and property of active sites in metal-containing zeolites. Moreover, detailed information on host-guest interactions in the relevant zeolite catalysis obtained by SSNMR is also discussed. Finally, we highlight the mechanistic understanding of catalytic reactions on metal-containing zeolites based on the observation of key surface species and active intermediates.
Keywordmetal-containing zeolites solid-state NMR active site host-guest interaction reaction mechanism
DOI10.1007/s11705-019-1885-1
WOS KeywordMODIFIED ZSM-5 ZEOLITES ; BRONSTED/LEWIS ACID SYNERGY ; C-13 CHEMICAL-SHIFT ; DEALUMINATED HY ZEOLITE ; TO-AROMATICS CONVERSION ; HOST-GUEST INTERACTIONS ; SN-BETA ZEOLITE ; MAS NMR ; PROPANE AROMATIZATION ; METHANOL CONVERSION
Language英语
WOS Research AreaEngineering
WOS SubjectEngineering, Chemical
WOS IDWOS:000522428600004
PublisherSPRINGER
Citation statistics
Cited Times:2[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.apm.ac.cn/handle/112942/22287
Collection中国科学院武汉物理与数学研究所
Corresponding AuthorXu, Jun; Deng, Feng
Affiliation1.Chinese Acad Sci, CAS Key Lab Magnet Resonance Biol Syst, Wuhan Inst Phys & Math,Innovat Acad Precis Measur, Natl Ctr Magnet Resonance Wuhan,State Key Lab Mag, Wuhan 430071, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Huazhong Univ Sci & Technol, Wuhan Natl Lab Optoelect, Wuhan 430074, Peoples R China
Recommended Citation
GB/T 7714
Zhao, Xingling,Xu, Jun,Deng, Feng. Solid-state NMR for metal-containing zeolites: From active sites to reaction mechanism[J]. FRONTIERS OF CHEMICAL SCIENCE AND ENGINEERING,2020,14(2):159-187.
APA Zhao, Xingling,Xu, Jun,&Deng, Feng.(2020).Solid-state NMR for metal-containing zeolites: From active sites to reaction mechanism.FRONTIERS OF CHEMICAL SCIENCE AND ENGINEERING,14(2),159-187.
MLA Zhao, Xingling,et al."Solid-state NMR for metal-containing zeolites: From active sites to reaction mechanism".FRONTIERS OF CHEMICAL SCIENCE AND ENGINEERING 14.2(2020):159-187.
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